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Spatiotemporal characteristics and diffusion flux of partial pressure of dissolved carbon dioxide (pCO2) in Hongjiadu reservoir.

YU Yuan-xiu1,3;LIU Cong-qiang1;WANG Fu-shun2;WANG Bao-li1;WANG Shi-lu1;LIU Fang1   

  1. 1State Key Laboratory of Environmental Geochemistry, Institute of Geoch
    emistry, Chinese Academy of Sciences, Guiyang 550002, China;2School of En
    vironmental and Chemical Engineering, Shanghai University, Shanghai 201800, China;3Graduate University of Chinese Academy of Sciences, Beijing 100039, China
  • Received:2008-01-10 Revised:1900-01-01 Online:2008-07-10 Published:2008-07-10

Abstract: In order to understand the characteristics of greenhouse gases emission from artificial reservoirs, the distribution characteristics of partial pressure of dissolved carbon dioxide (pCO2) in inflow waters, outflow waters, and the waters in Hongjiadu reservoir, a newly-built reservoir located in Guizhou Province of Southwest China, were analyzed in April, July and October 2006 and January 2007. The results showed that the pCO2 value in inflow waters was spring <summer<autumn<winter, and the annual average pCO2 in the inflow waters from Liuchong river and Washui river was 488 and 624 μatm, respectively. The pCO2 in reservoir epilimnion reached to the highest value (925 μatm) in winter and the lowest (279 μatm) in spring, with the annual average of 598 μatm. The pCO2 in water column increased with water depth. In the outflow waters, pCO2 was the highest (8 417 μatm) in summer and the lowest in winter (382 μatm), with the annual average value of 3 260 μatm. The annual average pCO2 in inflow waters, reservoir epilimnion, and outflow waters was higher than that of air (380 μatm pCO2), and the diffusion flux of CO2 at waterair interface was 3.93-6.29, 4.87-7.79 and 64.29-102.86 mmol·m-2·d-1, respectively, showing that the reservoir should be a CO2 source of the atmosphere. Through the action of the reservoir, the diffusion flux of CO2 was enhanced, with the pCO2 in outflow waters being 16 and 13 folds of that in inflow waters and reservoir epilimnion, respectively. Accordingly, much attention should be paid on the CO2 emission from the outflow waters of the reservoir.

Key words: Weibei dry upland, Apple planting subarea, Soil moisture characteristics, Dried soil layer